The Carbon Footprint of Radioactive Waste Immobilization - Abstract
From 1943 to 1989, the Hanford Nuclear Reservation produced weapons
grade plutonium and approximately 212,000 cubic meters of mixed radioactive and
hazardous chemical waste, filling 177 aging underground tanks. It is assumed that
90% of this waste is “Low Activity Waste” after cesium, strontium, and transuranics
are removed. In late 2025, the Direct Feed Low Activity Waste facility began
vitrification, i.e., mixing liquid waste with molten glass at 1150 °C, thereby destroying
hazardous organic chemicals. To continuously maintain heat in the two 300-ton melters,
approximately 200,000 megawatt-hours of electricity are required annually. Over
their 40-year lifetimes, these vitrification melters generate approximately 3,000,000
tonnes of carbon dioxide. This carbon footprint could be reduced by “grouting” a
substantial portion of the waste, i.e., mixing the waste with Portland cement, granulated
slag, and fly ash. In a recent agreement, the Washington State Department of Ecology
agreed in principle to grouting, provided that the resulting grout is shipped to a
dedicated off-site radioactive waste disposal facility. This would reduce Hanford’s
carbon footprint even after accounting for the CO2 from transportation.